Nanoscale Metrology Using the Spin and Charge States of Single Nitrogen Vacancy Centers in Diamond

Download or read book Nanoscale Metrology Using the Spin and Charge States of Single Nitrogen Vacancy Centers in Diamond written by Aedan Gardill and published by . This book was released on 2023 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: The nitrogen-vacancy (NV) center in diamond has shown great success as a nanoscale sensor due to its long coherence times at room temperature, its ability to be optically addressed, its sensitivity to a host of external fields, and having technical and logistical advantages due to being naturally trapped within the diamond. They have been used in a broad range of applications, including condensed matter physics, biology, geographical science, and commercial magnetometers. In this thesis, new nanoscale measurement techniques using single NV centers are presented that utilize their spin and charge states. First, the spin relaxation dynamics of single NV centers in nanodiamonds are measured, which sheds light on the electric noise spectral density of these nanodiamonds. Additionally, these measurements investigate the sources that limit coherence times of NV centers in nanodiamonds. Second, single NV centers are used to capture electrons released from surrounding defects in diamond in a new measurement technique. This allows us to gain new understanding of the charge dynamics of these surrounding defects. Lastly, a novel super-resolution technique is demonstrated with NV centers that uses the naturally formed Airy disk of light focused by a lens. This technique can be readily implemented in other confocal microscopes with little-to-no additional modifications. The NV center-based measurement techniques introduced in this thesis offer promising new measurement tools that could have large impacts in other research areas, such as quantum computing. For example, the electric field sensing technique could be used to explore the source of surface charge noise in materials used in superconducting qubits or semiconductor quantum dots. The work using single NV centers to probe charge dynamics also expands our understanding of the charge states of silicon vacancy centers in diamond, which are promising defects for quantum networks. Moreover, the demonstrated new super-resolution technique proves a gateway for other research groups to easily achieve super-resolution in their work and advance their research.